Manjula Perera

and 13 more

Inverse modelling method named Maximum likelihood Ensemble Filter (MLEF) was used to estimate gridded surface CO fluxes using continuous, flask and Comprehensive Observation Network for TRace gases by AIrLiner (CONTRAIL) data for the years 2009-2011. Here, MLEF coupled with Parametric Chemistry Transport Model (PCTM) driven by Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA2) weather data has been used. Flux estimation was done by solving separate multiplicative biases for photosynthesis, respiration, and air-sea gas exchange fluxes. Hourly land fluxes derived from Simple Biosphere-version 3 (SiB3) model, Takahashi ocean fluxes and Brenkert fossil fuel emissions were used as the prior fluxes. The inversion was carried out by assimilating hourly CO observations, According to this study, North America showed about 60-80% uncertainty reduction while the Asian and European regions showed moderate results with 50-60% uncertainty reduction. Most other land and oceanic regions showed less than 30% uncertainty reduction. The results were mainly compared with well-known CarbonTracker and some parallel inversion studies by considering long-term averages of the estimated fluxes for the TransCom regions. Boreal North America, Temperate North America and Australia showed similar annual averages in each case. Tropical Asia and Europe showed comparable results with all other studies except for the CarbonTracker. The biases were poorly constrained in the regions having few measurement sites like South America, Africa and Eurasian Temperate which showed completely different result with other studies.

Kenneth Davis

and 29 more

The Atmospheric Carbon and Transport (ACT) – America NASA Earth Venture Suborbital Mission set out to improve regional atmospheric greenhouse gas (GHG) inversions by exploring the intersection of the strong GHG fluxes and vigorous atmospheric transport that occurs within the midlatitudes. Two research aircraft instrumented with remote and in situ sensors to measure GHG mole fractions, associated trace gases, and atmospheric state variables collected 1140.7 flight hours of research data, distributed across 305 individual aircraft sorties, coordinated within 121 research flight days, and spanning five, six-week seasonal flight campaigns in the central and eastern United States. Flights sampled 31 synoptic sequences, including fair weather and frontal conditions, at altitudes ranging from the atmospheric boundary layer to the upper free troposphere. The observations were complemented with global and regional GHG flux and transport model ensembles. We found that midlatitude weather systems contain large spatial gradients in GHG mole fractions, in patterns that were consistent as a function of season and altitude. We attribute these patterns to a combination of regional terrestrial fluxes and inflow from the continental boundaries. These observations, when segregated according to altitude and air mass, provide a variety of quantitative insights into the realism of regional CO2 and CH4 fluxes and atmospheric GHG transport realizations. The ACT-America data set and ensemble modeling methods provide benchmarks for the development of atmospheric inversion systems. As global and regional atmospheric inversions incorporate ACT-America’s findings and methods, we anticipate these systems will produce increasingly accurate and precise sub-continental GHG flux estimates.

Sarah Gallup

and 6 more