An enhanced aerosol layer, known as the Asian Tropopause Aerosol Layer (ATAL), has been observed within the seasonal Asian monsoon anticyclone (AMA) since the late 1990s. Given the apparently abrupt appearance of this layer based on observations, it has been speculated that it originates from increasing human made emissions in Asia. However, the ATAL confinement is a result of a dynamical feature and does not purely consist of human made components. We herein investigate the possible existence of an ATAL earlier than the late 1990s. We exploit earliest possible, high quality space-based aerosol observations from Stratospheric Aerosol and Gas Experiment, or SAGE (1979-1981), SAGE III/ISS (2017, ongoing) and revisit SAGE II (1984-2005) data analysis. We find that seasonal averaged solar occultation aerosol measurements (past and present) can neither be used to exclude the existence of the ATAL, nor to infer a significant trend. However, first CAM5-MAM7 simulations indicate the presence of an ATAL signal for the tested years 1979 and 1980, with a human made component. We hypothesize that the human made component of the ATAL likely occurred since at least the 1970s, while the natural ATAL component (e.g. from dust) has always existed. Extended simulation based ATAL evolution studies are therefore the most reliable source for early ATAL investigations.

This study attempts to quantify the radiative impact over Reunion Island (21°S, 55°E) in the southern tropical Indian Ocean of the aerosols and water vapor injected in the stratosphere by the eruption on 15 January 2022 in the South Pacific of the Hunga Tonga-Hunga Ha’apai underwater volcano. Ground-based lidar and satellite passive instruments are used to parametrize a state-of-the-art radiative transfer model for the first thirteen months after the volcano eruption. The descending rate of the aerosol volcanic plume is -0.008 km day-1. At this rate, aerosols are expected to be present in the stratosphere until the first half of 2025. The overall aerosol and water vapor impact on the Earth’s radiation budget for the whole period is positive (warming, +0.06 ± 0.45 W m-2) and dominated by the aerosol impact. However, the decreasing rate with time of the aerosol warming effect is larger than that of the water vapor cooling effect, so that, in the long run, the impact on the Earth’s radiation budget might reduce to quasi-neutral, or even become slightly negative. At the Earth’s surface, aerosols are the main driver and produce a negative (cooling, -0.91 ± 0.61 W m-2) radiative impact with also a decreasing tendency with time. Heating/cooling rate profiles show a clear vertical difference in the stratosphere between the aerosol warming impact (17 to 25 km) and the water vapor cooling one (25 to 40 km).

The Hunga Tonga-Hunga Ha’apai volcano violently erupted on 15 January 2022, producing the largest perturbation of the stratospheric aerosol layer since Pinatubo 1991, despite the estimated modest injection of SO2. Here we present novel SO2 and sulphate aerosol (SA) co-retrievals from the Infrared Atmospheric Sounding Instrument, and use them to study the dispersion of the Hunga Tonga plume over the entire year 2022. We observe rapid conversion of SO2 (e-folding time: 17.1±0.6 days) to sulphate aerosols (SA), with an initial injected burden of >1.0 Tg. This points at larger SO2 injections than previously thought. A long-lasting SA plume was observed, with a meridional dispersion of marked anomalies from the tropics to the higher southern hemispheric latitudes. A very small SA removal is observed after 1-year dispersion. The total SA mass burden was estimated at 1.6 ± 0.1 Tg in total column, with a build-up e-folding time of about 2 months.

A document by Clair Duchamp. Click on the document to view its contents.

The eruption of the submarine Hunga volcano in January 2022 was associated with a powerful blast that injected volcanic material to altitudes up to 58 km. From a combination of various types of satellite and ground-based observations supported by transport modeling, we show evidence for an unprecedented increase in the global stratospheric water mass by 13% as compared to climatological levels, and a 5-fold increase of stratospheric aerosol load, the highest in the last three decades. Owing to the extreme injection altitude, the volcanic plume has circumnavigated the Earth in only one week and dispersed nearly pole-to-pole in three months. The unique nature and magnitude of the global stratospheric perturbation by the Hunga eruption ranks it among the most remarkable climatic events in the modern observation era, with a range of potential persistent repercussions for stratospheric composition and climate.

Following the Hunga Tonga eruption (20.6°S, 175.4°W, mid-January 2022), we present a balloon-borne characterization of the stratospheric aerosol plume one week after its injection (on 23 and 26/01/2022, La Réunion island at 21.1°S, 55.3°E). Satellite observations show that flight #1 took place during the overpass of a denser plume of sulfate aerosols (SA) compared to a more diluted plume during flight #2. Observations show that the sampled plumes (at around 22, 25 and 19 km altitude, respectively) consist exclusively of very small particles (with radius < 1 µm). Particles with radii between 0.5 and 1.0 µm show optically transparent features pointing to predominant SA. Particles with radii below 0.5 µm are partly absorbing, which could point to small sulfate coated ash particles, a feature not identified with space-borne observations. This shows that in situ observations are necessary to fully characterize the microphysical properties of the plumes tracked by space-borne instruments.